Telegraph Road.
The lead guitar, the dynamics, the plucked National throughout the verses, the synth, the piano, the organ. The storytelling lyrics perfectly corresponding with the dynamics in the music. The outtro. The vibe. The mood.
I still remember the day I first heard it, in May 1986. I had listened to the BiA and DS records hundreds of times already, but THAT way of playing guitar totally blew me away.